Efficient Dye-Sensitized Photovoltaic Wires Based on an Organic Redox Electrolyte

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State Key Laboratory of Molecular Engineering of Polymers, Department of Macromolecular Science, and Laboratory of Advanced Materials, Fudan University, Shanghai 200438, China
School of Materials Science and Engineering, Tongji University, 4800 Caoan Road, Shanghai 201804, China
Cite this: J. Am. Chem. Soc. 2013, 135, 29, 10622–10625
Publication Date (Web):July 15, 2013
https://doi.org/10.1021/ja405012w
Copyright © 2013 American Chemical Society
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Abstract

An organic thiolate/disulfide redox couple with low absorption in the visible region was developed for use in fabricating novel dye-sensitized photovoltaic wires with an aligned carbon nanotube (CNT) fiber as the counter electrode. These flexible wire devices achieved a maximal energy conversion efficiency of 7.33%, much higher than the value of 5.97% for the conventional I/I3 redox couple. In addition, the aligned CNT fiber also greatly outperforms the conventional Pt counter electrode with a maximal efficiency of 2.06% based on the thiolate/disulfide redox couple.

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Synthesis of the organic electrolyte and structure and property characterizations of devices. This material is available free of charge via the Internet at http://pubs.acs.org.

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